Electronically Driven Fragmentation of Silver Nanocrystals Revealed by Ultrafast Electron Crystallography

We report an ultrafast electron diffraction study of silver nanocrystals under surface plasmon resonance excitation, leading to a concerted fragmentation. By examining simultaneously transient structural, thermal, and Coulombic signatures of the prefragmented state, an electronically driven nontherm...

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Veröffentlicht in:	arXiv.org 2013-09
Hauptverfasser:	Raman, Ramani K, Murdick, Ryan A, Worhatch, Richard J, Murooka, Yoshie, Mahanti, Subhendra D, Han, Tzong-Ru T, Chong-Yu, Ruan
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Sprache:	eng
Schlagworte:	Crystallography Electron diffraction Fragmentation Nanocrystals Physics - Materials Science
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creator	Raman, Ramani K Murdick, Ryan A Worhatch, Richard J Murooka, Yoshie Mahanti, Subhendra D Han, Tzong-Ru T Chong-Yu, Ruan
description	We report an ultrafast electron diffraction study of silver nanocrystals under surface plasmon resonance excitation, leading to a concerted fragmentation. By examining simultaneously transient structural, thermal, and Coulombic signatures of the prefragmented state, an electronically driven nonthermal fragmentation scenario is proposed.
doi_str_mv	10.48550/arxiv.1309.3351
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subjects	Crystallography Electron diffraction Fragmentation Nanocrystals Physics - Materials Science
title	Electronically Driven Fragmentation of Silver Nanocrystals Revealed by Ultrafast Electron Crystallography
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