Observation of Coulomb-Assisted Dipole-Forbidden Intraexciton Transitions in Semiconductors
We use terahertz pulses to induce resonant transitions between the eigenstates of optically generated exciton populations in a high-quality semiconductor quantum-well sample. Monitoring the excitonic photoluminescence, we observe transient quenching of the \(1s\) exciton emission, which we attribute...
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creator | Rice, W D Kono, J Zybell, S Winnerl, S Bhattacharyya, J Schneider, H Helm, M Ewers, B Chernikov, A Koch, M Chatterjee, S Khitrova, G Gibbs, H M Schneebeli, L Breddermann, B Kira, M Koch, S W |
description | We use terahertz pulses to induce resonant transitions between the eigenstates of optically generated exciton populations in a high-quality semiconductor quantum-well sample. Monitoring the excitonic photoluminescence, we observe transient quenching of the \(1s\) exciton emission, which we attribute to the terahertz-induced \(1s\)-to-\(2p\) excitation. Simultaneously, a pronounced enhancement of the \(2s\)-exciton emission is observed, despite the \(1s\)-to-\(2s\) transition being dipole forbidden. A microscopic many-body theory explains the experimental observations as a Coulomb-scattering mixing of the 2\(s\) and 2\(p\) states, yielding an effective terahertz transition between the 1\(s\) and 2\(s\) populations. |
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Monitoring the excitonic photoluminescence, we observe transient quenching of the \(1s\) exciton emission, which we attribute to the terahertz-induced \(1s\)-to-\(2p\) excitation. Simultaneously, a pronounced enhancement of the \(2s\)-exciton emission is observed, despite the \(1s\)-to-\(2s\) transition being dipole forbidden. A microscopic many-body theory explains the experimental observations as a Coulomb-scattering mixing of the 2\(s\) and 2\(p\) states, yielding an effective terahertz transition between the 1\(s\) and 2\(s\) populations.</description><identifier>EISSN: 2331-8422</identifier><identifier>DOI: 10.48550/arxiv.1203.3994</identifier><language>eng</language><publisher>Ithaca: Cornell University Library, arXiv.org</publisher><subject>Dipoles ; Eigenvectors ; Emission ; Excitons ; Photoluminescence ; Physics - Mesoscale and Nanoscale Physics ; Populations ; Quantum wells</subject><ispartof>arXiv.org, 2012-12</ispartof><rights>2012. 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Monitoring the excitonic photoluminescence, we observe transient quenching of the \(1s\) exciton emission, which we attribute to the terahertz-induced \(1s\)-to-\(2p\) excitation. Simultaneously, a pronounced enhancement of the \(2s\)-exciton emission is observed, despite the \(1s\)-to-\(2s\) transition being dipole forbidden. A microscopic many-body theory explains the experimental observations as a Coulomb-scattering mixing of the 2\(s\) and 2\(p\) states, yielding an effective terahertz transition between the 1\(s\) and 2\(s\) populations.</description><subject>Dipoles</subject><subject>Eigenvectors</subject><subject>Emission</subject><subject>Excitons</subject><subject>Photoluminescence</subject><subject>Physics - Mesoscale and Nanoscale Physics</subject><subject>Populations</subject><subject>Quantum wells</subject><issn>2331-8422</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2012</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><sourceid>GOX</sourceid><recordid>eNotkD1rwzAYhEWh0JBm71QMne2--nKkMbhNGwhkaLYORpZkUIglV7JD-u8bJ51uuee4O4SeMBRMcA6vKp7dqcAEaEGlZHdoRijFuWCEPKBFSgcAIOWScE5n6HvXJBtPanDBZ6HNqjAeQ9fkq5RcGqzJ3lwfjjZfh9g4Y6zPNn6Iyp61Gy7EPiqf3ASnzPnsy3ZOB29GPYSYHtF9q47JLv51jvbr9331mW93H5tqtc0Vx5BbjUVZEsGNMFoqLY1SbamAMM6YkVxr1toGE8IMFxqWjAJgaEHKRrKGLOkcPd9ir8PrPrpOxd96OqCeDrgYXm6GPoaf0aahPoQx-kulmoDglHNZAv0DL8pe_g</recordid><startdate>20121205</startdate><enddate>20121205</enddate><creator>Rice, W D</creator><creator>Kono, J</creator><creator>Zybell, S</creator><creator>Winnerl, S</creator><creator>Bhattacharyya, J</creator><creator>Schneider, H</creator><creator>Helm, M</creator><creator>Ewers, B</creator><creator>Chernikov, A</creator><creator>Koch, M</creator><creator>Chatterjee, S</creator><creator>Khitrova, G</creator><creator>Gibbs, H M</creator><creator>Schneebeli, L</creator><creator>Breddermann, B</creator><creator>Kira, M</creator><creator>Koch, S W</creator><general>Cornell University Library, arXiv.org</general><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>L6V</scope><scope>M7S</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PTHSS</scope><scope>GOX</scope></search><sort><creationdate>20121205</creationdate><title>Observation of Coulomb-Assisted Dipole-Forbidden Intraexciton Transitions in Semiconductors</title><author>Rice, W D ; 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subjects | Dipoles Eigenvectors Emission Excitons Photoluminescence Physics - Mesoscale and Nanoscale Physics Populations Quantum wells |
title | Observation of Coulomb-Assisted Dipole-Forbidden Intraexciton Transitions in Semiconductors |
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