Thermal expansion of the magnetically ordering intermetallics RTMg (R = Eu, Gd and T = Ag, Au)

We report measurements of the thermal expansion for two Eu\(^{+2}\)- and two Gd\(^{+3}\)-based intermetallics which exhibit ferro- or antiferromagnetic phase transitions. These materials show sharp positive (EuAgMg and GdAuMg) and negative (EuAuMg and GdAgMg) peaks in the temperature dependence of t...

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Veröffentlicht in:arXiv.org 2007-08
Hauptverfasser: Rohrkamp, J, Heyer, O, Fickenscher, T, Poettgen, R, Jodlauk, S, Hartmann, H, Lorenz, T, Mydosh, J A
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creator Rohrkamp, J
Heyer, O
Fickenscher, T
Poettgen, R
Jodlauk, S
Hartmann, H
Lorenz, T
Mydosh, J A
description We report measurements of the thermal expansion for two Eu\(^{+2}\)- and two Gd\(^{+3}\)-based intermetallics which exhibit ferro- or antiferromagnetic phase transitions. These materials show sharp positive (EuAgMg and GdAuMg) and negative (EuAuMg and GdAgMg) peaks in the temperature dependence of the thermal expansion coefficient \(\alpha\) which become smeared and/or displaced in an external magnetic field. Together with specific heat data we determine the initial pressure dependences of the transition temperatures at ambient pressure using the Ehrenfest or Clausius-Clapeyron relation. We find large pressure dependences indicating strong spin-phonon coupling, in particular for GdAgMg and EuAuMg where a quantum phase transition might be reached at moderate pressures of a few GPa.
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subjects Antiferromagnetism
Gadolinium
Gold
Initial pressure
Intermetallic compounds
Phase transitions
Physics - Materials Science
Physics - Other Condensed Matter
Pressure
Silver
Temperature
Temperature dependence
Thermal expansion
title Thermal expansion of the magnetically ordering intermetallics RTMg (R = Eu, Gd and T = Ag, Au)
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