Real-Time, Selective Detection of Pb2+ in Water Using a Reduced Graphene Oxide/Gold Nanoparticle Field-Effect Transistor Device
A field-effect transistor (FET) device-based sensor is developed to specifically detect Pb2+ ions in an aqueous environment that is notably toxic. Reduced graphene oxide (rGO), as the semiconducting channel material, was utilized in the FET device through a self-assembly method. An l-glutathione red...
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Veröffentlicht in: | ACS applied materials & interfaces 2014-11, Vol.6 (21), p.19235-19241 |
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creator | Zhou, Guihua Chang, Jingbo Cui, Shumao Pu, Haihui Wen, Zhenhai Chen, Junhong |
description | A field-effect transistor (FET) device-based sensor is developed to specifically detect Pb2+ ions in an aqueous environment that is notably toxic. Reduced graphene oxide (rGO), as the semiconducting channel material, was utilized in the FET device through a self-assembly method. An l-glutathione reduced was employed as the capture probe for the label-free detection. By monitoring the electrical characteristics of the FET device, the performance of the sensor was measured and investigated. Compared with conventional detection technologies, this sensor enabled real-time detection with a response time of 1–2 s. A lower detection limit for Pb2+ ions as low as 10 nM was achieved, which is much lower than the maximum contaminant level for Pb2+ ions in drinking water recommended by the World Health Organization. Furthermore, the rGO FET sensor was able to distinguish Pb2+ from other metal ions. Without any sample pretreatment, the platform is user-friendly. |
doi_str_mv | 10.1021/am505275a |
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Reduced graphene oxide (rGO), as the semiconducting channel material, was utilized in the FET device through a self-assembly method. An l-glutathione reduced was employed as the capture probe for the label-free detection. By monitoring the electrical characteristics of the FET device, the performance of the sensor was measured and investigated. Compared with conventional detection technologies, this sensor enabled real-time detection with a response time of 1–2 s. A lower detection limit for Pb2+ ions as low as 10 nM was achieved, which is much lower than the maximum contaminant level for Pb2+ ions in drinking water recommended by the World Health Organization. Furthermore, the rGO FET sensor was able to distinguish Pb2+ from other metal ions. 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Mater. Interfaces</addtitle><description>A field-effect transistor (FET) device-based sensor is developed to specifically detect Pb2+ ions in an aqueous environment that is notably toxic. Reduced graphene oxide (rGO), as the semiconducting channel material, was utilized in the FET device through a self-assembly method. An l-glutathione reduced was employed as the capture probe for the label-free detection. By monitoring the electrical characteristics of the FET device, the performance of the sensor was measured and investigated. Compared with conventional detection technologies, this sensor enabled real-time detection with a response time of 1–2 s. A lower detection limit for Pb2+ ions as low as 10 nM was achieved, which is much lower than the maximum contaminant level for Pb2+ ions in drinking water recommended by the World Health Organization. Furthermore, the rGO FET sensor was able to distinguish Pb2+ from other metal ions. 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Mater. Interfaces</addtitle><date>2014-11-12</date><risdate>2014</risdate><volume>6</volume><issue>21</issue><spage>19235</spage><epage>19241</epage><pages>19235-19241</pages><issn>1944-8244</issn><eissn>1944-8252</eissn><abstract>A field-effect transistor (FET) device-based sensor is developed to specifically detect Pb2+ ions in an aqueous environment that is notably toxic. Reduced graphene oxide (rGO), as the semiconducting channel material, was utilized in the FET device through a self-assembly method. An l-glutathione reduced was employed as the capture probe for the label-free detection. By monitoring the electrical characteristics of the FET device, the performance of the sensor was measured and investigated. Compared with conventional detection technologies, this sensor enabled real-time detection with a response time of 1–2 s. A lower detection limit for Pb2+ ions as low as 10 nM was achieved, which is much lower than the maximum contaminant level for Pb2+ ions in drinking water recommended by the World Health Organization. Furthermore, the rGO FET sensor was able to distinguish Pb2+ from other metal ions. Without any sample pretreatment, the platform is user-friendly.</abstract><pub>American Chemical Society</pub><doi>10.1021/am505275a</doi><tpages>7</tpages></addata></record> |
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title | Real-Time, Selective Detection of Pb2+ in Water Using a Reduced Graphene Oxide/Gold Nanoparticle Field-Effect Transistor Device |
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