Screen-Printing Preparation of High-Performance Nonenzymatic Glucose Sensors Based on Co3O4 Nanoparticles-Embedded N‑Doped Laser-Induced Graphene

Screen-Printing Preparation of High-Performance Nonenzymatic Glucose Sensors Based on Co3O4 Nanoparticles-Embedded N‑Doped Laser-Induced Graphene

Precise acquisition of the blood glucose level is one of the most critical indicators for the prevention and treatment of diabetes. Compared with the high cost and instability of enzyme-based glucose sensors, the development of low-cost, high-sensitivity, and fast-response nonenzymatic glucose senso...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:ACS applied nano materials 2022-11, Vol.5 (11), p.16655-16663
Hauptverfasser: Li, Chen, Xiong, Jijun, Zheng, Caidong, Zhao, Jiang
Format: Artikel
Sprache:eng
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 16663
container_issue 11
container_start_page 16655
container_title ACS applied nano materials
container_volume 5
creator Li, Chen
Xiong, Jijun
Zheng, Caidong
Zhao, Jiang
description Precise acquisition of the blood glucose level is one of the most critical indicators for the prevention and treatment of diabetes. Compared with the high cost and instability of enzyme-based glucose sensors, the development of low-cost, high-sensitivity, and fast-response nonenzymatic glucose sensors is imperative. Herein, bulk Co3O4-embedded N-doped laser-induced graphene (Co3O4@NLIG) powder is in situ fabricated through a high-efficiency and simple laser-scribing technique and successfully made into a screen-printing paste for screen-printed electrodes (SPEs), followed by use as an enzyme-free glucose sensor. The electrocatalytic results show that the as-prepared Co3O4@NLIG/SPE glucose sensor has a high sensitivity of 143 μA mM–1 cm–2, a broad linear detection range of 1 μM to 11 mM, an ultralow detection limit of 0.48 μM, and a rapid response time of
doi_str_mv 10.1021/acsanm.2c03694
format Article
fullrecord <record><control><sourceid>acs</sourceid><recordid>TN_cdi_acs_journals_10_1021_acsanm_2c03694</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>a213710915</sourcerecordid><originalsourceid>FETCH-LOGICAL-a120t-568f4644b7907e5e45841bb914df193433f2a3ca7ffc4a5f9dcdb5ecf405efd13</originalsourceid><addsrcrecordid>eNpNkEFPAjEQhRujiQS5eu7ZpNhuu7v0qIhAQoAEPW-67RSWsC1p4aAn_oLxH_pLrIGDp3mTefNe8iF0z2if0Yw9Kh2Va_uZpryQ4gp1srwUhMqSXv_Tt6gX45ZSyiQrOKUd9L3SAcCRZWjcoXFrvAywV0EdGu-wt3jSrDdkCcH60CqnAc-9A_f50SaHxuPdUfsIeAUu-hDxs4pgcPocer4QeK6cT2HJuYNIRm0NxqT7_Of09eL3Sc2SP5CpM0edtnFQ-w04uEM3Vu0i9C6zi95fR2_DCZktxtPh04woltEDyYuBFYUQdSlpCTmIfCBYXUsmjGWSC85tprhWpbVaqNxKo02dg7aC5mAN4130cM5N8KqtPwaX2ipGqz-i1ZlodSHKfwGyIW4K</addsrcrecordid><sourcetype>Publisher</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Screen-Printing Preparation of High-Performance Nonenzymatic Glucose Sensors Based on Co3O4 Nanoparticles-Embedded N‑Doped Laser-Induced Graphene</title><source>ACS Publications</source><creator>Li, Chen ; Xiong, Jijun ; Zheng, Caidong ; Zhao, Jiang</creator><creatorcontrib>Li, Chen ; Xiong, Jijun ; Zheng, Caidong ; Zhao, Jiang</creatorcontrib><description>Precise acquisition of the blood glucose level is one of the most critical indicators for the prevention and treatment of diabetes. Compared with the high cost and instability of enzyme-based glucose sensors, the development of low-cost, high-sensitivity, and fast-response nonenzymatic glucose sensors is imperative. Herein, bulk Co3O4-embedded N-doped laser-induced graphene (Co3O4@NLIG) powder is in situ fabricated through a high-efficiency and simple laser-scribing technique and successfully made into a screen-printing paste for screen-printed electrodes (SPEs), followed by use as an enzyme-free glucose sensor. The electrocatalytic results show that the as-prepared Co3O4@NLIG/SPE glucose sensor has a high sensitivity of 143 μA mM–1 cm–2, a broad linear detection range of 1 μM to 11 mM, an ultralow detection limit of 0.48 μM, and a rapid response time of &lt;1 s. The as-prepared sensor also has prominent reproducibility, stability, and immunity to interference. Furthermore, the glucose-sensing mechanism of the sensor is profoundly explored. Such an outstanding electrocatalytic performance endows the Co3O4@NLIG/SPE nonenzymatic glucose sensor with potential applications in blood glucose monitoring and diagnosis.</description><identifier>ISSN: 2574-0970</identifier><identifier>EISSN: 2574-0970</identifier><identifier>DOI: 10.1021/acsanm.2c03694</identifier><language>eng</language><publisher>American Chemical Society</publisher><ispartof>ACS applied nano materials, 2022-11, Vol.5 (11), p.16655-16663</ispartof><rights>2022 American Chemical Society</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><orcidid>0000-0002-4098-5786</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/acsanm.2c03694$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/acsanm.2c03694$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,776,780,27055,27903,27904,56717,56767</link.rule.ids></links><search><creatorcontrib>Li, Chen</creatorcontrib><creatorcontrib>Xiong, Jijun</creatorcontrib><creatorcontrib>Zheng, Caidong</creatorcontrib><creatorcontrib>Zhao, Jiang</creatorcontrib><title>Screen-Printing Preparation of High-Performance Nonenzymatic Glucose Sensors Based on Co3O4 Nanoparticles-Embedded N‑Doped Laser-Induced Graphene</title><title>ACS applied nano materials</title><addtitle>ACS Appl. Nano Mater</addtitle><description>Precise acquisition of the blood glucose level is one of the most critical indicators for the prevention and treatment of diabetes. Compared with the high cost and instability of enzyme-based glucose sensors, the development of low-cost, high-sensitivity, and fast-response nonenzymatic glucose sensors is imperative. Herein, bulk Co3O4-embedded N-doped laser-induced graphene (Co3O4@NLIG) powder is in situ fabricated through a high-efficiency and simple laser-scribing technique and successfully made into a screen-printing paste for screen-printed electrodes (SPEs), followed by use as an enzyme-free glucose sensor. The electrocatalytic results show that the as-prepared Co3O4@NLIG/SPE glucose sensor has a high sensitivity of 143 μA mM–1 cm–2, a broad linear detection range of 1 μM to 11 mM, an ultralow detection limit of 0.48 μM, and a rapid response time of &lt;1 s. The as-prepared sensor also has prominent reproducibility, stability, and immunity to interference. Furthermore, the glucose-sensing mechanism of the sensor is profoundly explored. Such an outstanding electrocatalytic performance endows the Co3O4@NLIG/SPE nonenzymatic glucose sensor with potential applications in blood glucose monitoring and diagnosis.</description><issn>2574-0970</issn><issn>2574-0970</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid/><recordid>eNpNkEFPAjEQhRujiQS5eu7ZpNhuu7v0qIhAQoAEPW-67RSWsC1p4aAn_oLxH_pLrIGDp3mTefNe8iF0z2if0Yw9Kh2Va_uZpryQ4gp1srwUhMqSXv_Tt6gX45ZSyiQrOKUd9L3SAcCRZWjcoXFrvAywV0EdGu-wt3jSrDdkCcH60CqnAc-9A_f50SaHxuPdUfsIeAUu-hDxs4pgcPocer4QeK6cT2HJuYNIRm0NxqT7_Of09eL3Sc2SP5CpM0edtnFQ-w04uEM3Vu0i9C6zi95fR2_DCZktxtPh04woltEDyYuBFYUQdSlpCTmIfCBYXUsmjGWSC85tprhWpbVaqNxKo02dg7aC5mAN4130cM5N8KqtPwaX2ipGqz-i1ZlodSHKfwGyIW4K</recordid><startdate>20221125</startdate><enddate>20221125</enddate><creator>Li, Chen</creator><creator>Xiong, Jijun</creator><creator>Zheng, Caidong</creator><creator>Zhao, Jiang</creator><general>American Chemical Society</general><scope/><orcidid>https://orcid.org/0000-0002-4098-5786</orcidid></search><sort><creationdate>20221125</creationdate><title>Screen-Printing Preparation of High-Performance Nonenzymatic Glucose Sensors Based on Co3O4 Nanoparticles-Embedded N‑Doped Laser-Induced Graphene</title><author>Li, Chen ; Xiong, Jijun ; Zheng, Caidong ; Zhao, Jiang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a120t-568f4644b7907e5e45841bb914df193433f2a3ca7ffc4a5f9dcdb5ecf405efd13</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Chen</creatorcontrib><creatorcontrib>Xiong, Jijun</creatorcontrib><creatorcontrib>Zheng, Caidong</creatorcontrib><creatorcontrib>Zhao, Jiang</creatorcontrib><jtitle>ACS applied nano materials</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Chen</au><au>Xiong, Jijun</au><au>Zheng, Caidong</au><au>Zhao, Jiang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Screen-Printing Preparation of High-Performance Nonenzymatic Glucose Sensors Based on Co3O4 Nanoparticles-Embedded N‑Doped Laser-Induced Graphene</atitle><jtitle>ACS applied nano materials</jtitle><addtitle>ACS Appl. Nano Mater</addtitle><date>2022-11-25</date><risdate>2022</risdate><volume>5</volume><issue>11</issue><spage>16655</spage><epage>16663</epage><pages>16655-16663</pages><issn>2574-0970</issn><eissn>2574-0970</eissn><abstract>Precise acquisition of the blood glucose level is one of the most critical indicators for the prevention and treatment of diabetes. Compared with the high cost and instability of enzyme-based glucose sensors, the development of low-cost, high-sensitivity, and fast-response nonenzymatic glucose sensors is imperative. Herein, bulk Co3O4-embedded N-doped laser-induced graphene (Co3O4@NLIG) powder is in situ fabricated through a high-efficiency and simple laser-scribing technique and successfully made into a screen-printing paste for screen-printed electrodes (SPEs), followed by use as an enzyme-free glucose sensor. The electrocatalytic results show that the as-prepared Co3O4@NLIG/SPE glucose sensor has a high sensitivity of 143 μA mM–1 cm–2, a broad linear detection range of 1 μM to 11 mM, an ultralow detection limit of 0.48 μM, and a rapid response time of &lt;1 s. The as-prepared sensor also has prominent reproducibility, stability, and immunity to interference. Furthermore, the glucose-sensing mechanism of the sensor is profoundly explored. Such an outstanding electrocatalytic performance endows the Co3O4@NLIG/SPE nonenzymatic glucose sensor with potential applications in blood glucose monitoring and diagnosis.</abstract><pub>American Chemical Society</pub><doi>10.1021/acsanm.2c03694</doi><tpages>9</tpages><orcidid>https://orcid.org/0000-0002-4098-5786</orcidid></addata></record>
fulltext fulltext
identifier ISSN: 2574-0970
ispartof ACS applied nano materials, 2022-11, Vol.5 (11), p.16655-16663
issn 2574-0970
2574-0970
language eng
recordid cdi_acs_journals_10_1021_acsanm_2c03694
source ACS Publications
title Screen-Printing Preparation of High-Performance Nonenzymatic Glucose Sensors Based on Co3O4 Nanoparticles-Embedded N‑Doped Laser-Induced Graphene
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-23T05%3A17%3A20IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-acs&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Screen-Printing%20Preparation%20of%20High-Performance%20Nonenzymatic%20Glucose%20Sensors%20Based%20on%20Co3O4%20Nanoparticles-Embedded%20N%E2%80%91Doped%20Laser-Induced%20Graphene&rft.jtitle=ACS%20applied%20nano%20materials&rft.au=Li,%20Chen&rft.date=2022-11-25&rft.volume=5&rft.issue=11&rft.spage=16655&rft.epage=16663&rft.pages=16655-16663&rft.issn=2574-0970&rft.eissn=2574-0970&rft_id=info:doi/10.1021/acsanm.2c03694&rft_dat=%3Cacs%3Ea213710915%3C/acs%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true